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A novel, exfoliating hydrogel was designed to achieve local drug delivery at different skin depths. Within the gel, the hydrophilic BODIPY fluorophores are partially encapsulated and maintain a low fluorescence, as a result of π-π stacking interactions with the hydrophobic triphenylphosphonium cation. Unlike most encapsulation procedures, which rely on simple dispersing of the fluorophore in a hydrophobic vehicle, the system is based on the initial loading of the fluorophores into a hydrophilic environment. It is also pH-responsive, to exert local treatment within the mildly acidic environment of the stratum corneum and the acidic environment of the hair follicle. In vitro experiments with freshly isolated pig scales confirm the penetration of the polymer into the stratum corneum and follicles at an acidic pH, whereas normal skin at the same pH does not permit the penetration of the gel into deep skin layers. After topical application of the gel, the individual fluorophores are released in a pH-dependent manner as the polymer breaks down and the hydrophobic fluorophores are released from the gel matrix. Confocal imaging of the treated live skin shows the penetration of the exfoliating gel into the hair follicles of the skin.Q:
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